浅谈碳酸盐分解耦合CO2原位还原技术国内外研究进展

doi:10.19698/j.cnki.1001-6171.20253002

下载:

PDF (10019KB)
输出: BibTeX | EndNote (RIS)

摘要探讨了甲烷干重整（CH₄-DRM）与碳酸盐分解技术协同应用于水泥行业CO₂减排的潜力及工业应用前景。介绍了CH₄-DRM反应的基本原理及热力学特性，分析了其在CO₂资源化利用中的关键作用，并总结了相关催化剂设计和反应条件优化的研究进展。对于碳酸盐分解的原位CO₂还原，探讨了其热效率优势及与CH₄-DRM的工业耦合路径，评估了工业化应用的可行性。最后，从明晰反应机理、工艺整合、催化剂优化和规模化利用评估等方面提出了未来研究方向，为水泥行业低碳转型提供理论支持和技术指导。

	服务
	把本文推荐给朋友
	加入引用管理器
	E-mail Alert
	RSS
	（）
	作者相关文章
	赵琳
	赵亮
	王佳硕
	杨欢迎

关键词: 碳酸盐分解耦合 CH₄干重整 Ni基催化剂 CO₂减排 CO₂资源化利用

Abstract: This paper discusses the potential of synergistic application of methane dry reforming (CH₄-DRM) and carbonate decomposition technology for CO₂ emission reduction in the cement industry and its industrial application prospects. The basic principle and thermodynamic characteristics of CH₄-DRM reaction are introduced, and its key role in CO₂ resource utilization is analyzed. The research progress of related catalyst design and reaction condition optimization is also summarized. For in-situ CO₂ reduction via carbonate decomposition, the thermal efficiency advantages and the industrial coupling approaches with CH₄-DRM are discussed, and the feasibility of industrial application is evaluated. Finally, the future research directions are proposed based on clarifying reaction mechanism, process integration, catalyst optimization and large-scale utilization evaluation, providing theoretical support and technical guidance for the low-carbon transformation of the cement industry.

Key words: carbonate decomposition coupling CH₄ dry reforming Ni-based catalyst CO₂ emission reduction CO₂ resource utilization

收稿日期: 2025-02-19 出版日期: 2025-05-25 发布日期: 2025-05-25 整期出版日期: 2025-05-25

ZTFLH:

X701.7

基金资助: 国家重点研发计划项目（2022YFA1504700）

作者简介: 赵琳（1989—），女，博士，高级工程师，主要从事大气污染物净化技术及材料的研究。E-mail:zhaolin3@sinoma-tianjin.cn

引用本文:

赵琳, 赵亮, 王佳硕, 杨欢迎. 浅谈碳酸盐分解耦合CO2原位还原技术国内外研究进展[J]. 水泥技术, 2025, 1(3): 2-10.
ZHAO Lin, ZHAO Liang, WANG Jiashuo, YANG Huanying. The Research Progress of Carbonate Decomposition Coupled with CO₂ In-situ Reduction Technology at Home and Abroad. Cement Technology, 2025, 1(3): 2-10.

链接本文:

http://www.cemteck.com/CN/10.19698/j.cnki.1001-6171.20253002 或 http://www.cemteck.com/CN/Y2025/V1/I3/2

[1]	. Review and Prospect of Engineering Practice of Waste Disposal in Cement Kiln in China[J]. Cement Technology, 2018, 1(1): 17 -21 .
[2]	DI Dongren, TAO Congxi, CHAI Xingteng. Revision of Cement Energy Consumption Standards and Energy Saving Technology(Ⅰ)[J]. Cement Technology, 2018, 1(1): 22 -26 .
[3]	LIU Yonggang, GAO Hongwei, XIAO Guiqing. Design Method of Road Structure Using Lean Concrete Base[J]. Cement Technology, 2018, 1(1): 27 -31 .
[4]	LIU Xu, LI Liang. Investigation of New Medium Temperature Wear-resistant Alloy Steel[J]. Cement Technology, 2018, 1(1): 32 -34 .
[5]	MA Debao. Finite Element Analysis of Inverted Cone in Raw Meal Silo[J]. Cement Technology, 2018, 1(1): 35 -38 .
[6]	HAN Zhongqi. [J]. Cement Technology, 2018, 1(1): 38 -48 .
[7]	XIE Jianzhong, LIAN Xuewen. Analysis and Solution of Segregation of the Kiln Ash in Continuous Raw Meal Homogenization Silo#br#[J]. Cement Technology, 2018, 1(1): 49 -53 .
[8]	GUAN Laiqing, HE Yongxian. [J]. Cement Technology, 2018, 1(1): 54 -59 .
[9]	WEI Can, ZHANG Yuanyuan, AI Jun. Application of Cement Intelligent Control System in Overseas Projects[J]. Cement Technology, 2018, 1(1): 60 -64 .
[10]	JIN Shuang. [J]. Cement Technology, 2018, 1(1): 72 -73 .